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GreatFET One
A Python-programmable USB peripheral tool.
Pins
The major attraction of the GreatFET is its array of I/O pins. The main headers (J1, J2, J7) contain 100 pins total, a few of which are set aside for special protocols.
All I/O pins on the GreatFET are 3.3 V only! Do not attempt to use with 5 V logic.
Right now, the best sources of pinout information are https://gf.ktemkin.com/ and https://github.com/greatfet-hardware/azalea.
CLI
The greatfet
Python package includes a series of CLI scripts for working with the various interfaces.